Abstract

Abstract The escalating level of atmospheric carbon dioxide is one of the most pressing environmental concerns of our age. Carbon capture and storage (CCS) from large point sources such as power plants is one option for reducing anthropogenic CO 2 emissions; however, currently the capture alone will increase the energy requirements of a plant by 25–40 %. This Review highlights the challenges for capture technologies which have the greatest likelihood of reducing CO 2 emissions to the atmosphere, namely postcombustion (predominantly CO 2 /N 2 separation), precombustion (CO 2 /H 2 ) capture, and natural gas sweetening (CO 2 /CH 4 ). The key factor which underlies significant advancements lies in improved materials that perform the separations. In this regard, the most recent developments and emerging concepts in CO 2 separations by solvent absorption, chemical and physical adsorption, and membranes, amongst others, will be discussed, with particular attention on progress in the burgeoning field of metal–organic frameworks.

Keywords

SweeteningCarbon dioxideEnvironmental scienceCarbon dioxide in Earth's atmosphereCarbon capture and storage (timeline)Process engineeringAtmosphere (unit)Waste managementEnvironmental chemistryChemistryEngineeringMeteorologyPhysics

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Publication Info

Year
2010
Type
article
Volume
49
Issue
35
Pages
6058-6082
Citations
3910
Access
Closed

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Deanna M. D’Alessandro, Berend Smit, Jeffrey R. Long (2010). Carbon Dioxide Capture: Prospects for New Materials. Angewandte Chemie International Edition , 49 (35) , 6058-6082. https://doi.org/10.1002/anie.201000431

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DOI
10.1002/anie.201000431