Abstract

Optical second harmonic spectroscopy is introduced as a powerful supplement for the determination of complex magnetic structures. Experimental efforts are simplified and new degrees of freedom are opened. Thereby, some principal or technical restrictions of neutron or magnetic x-ray diffraction experiments are overcome. High spatial resolution leads to additional information about magnetically ordered matter. As an example, the noncollinear magnetic structure of the hexagonal manganites RMnO3 ( R = Sc, Y, Ho, Er, Tm, Yb, Lu) is analyzed. The results show that some earlier conclusions on their magnetic symmetry and properties should be revised.

Keywords

Symmetry (geometry)Hexagonal crystal systemCondensed matter physicsMagnetic structurePhysicsDiffractionMaterials scienceSecond-harmonic generationHarmonicOpticsMagnetizationMagnetic fieldQuantum mechanicsCrystallographyChemistry

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Publication Info

Year
2000
Type
article
Volume
84
Issue
24
Pages
5620-5623
Citations
328
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Closed

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M. Fiebig, D. Fröhlich, Kay Kohn et al. (2000). Determination of the Magnetic Symmetry of Hexagonal Manganites by Second Harmonic Generation. Physical Review Letters , 84 (24) , 5620-5623. https://doi.org/10.1103/physrevlett.84.5620

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DOI
10.1103/physrevlett.84.5620