Abstract

By using a three-dimensional time-dependent Schr\"odinger equation, we calculate alignment-dependent ionization of model diatomic molecules subjected to an intense laser field with different internuclear distances. It is found that the ionization probability shows oscillatory behavior with respect to the angle between the laser polarization direction and the molecular axis for large internuclear distances. Comparing with the results obtained by Ammosov--Delone--Krainov (ADK) theory and $S$-matrix theory, the intriguing phenomenon can be attributed to the two-center interference effect of low-energy photoelectrons. Furthermore, it is shown that ADK theory is not applicable for the investigation of molecular ionization for large internuclear distances.

Keywords

ElectronAtomic physicsIonizationInterference (communication)PhysicsEnergy (signal processing)Electron ionizationNuclear physicsIonQuantum mechanicsChannel (broadcasting)

Affiliated Institutions

Related Publications

A Simplification of the Hartree-Fock Method

It is shown that the Hartree-Fock equations can be regarded as ordinary Schr\"odinger equations for the motion of electrons, each electron moving in a slightly different potenti...

1951 Physical Review 4470 citations

Surface-enhanced Raman scattering

On the basis of different types of experiments, the authors develop implicitly the model of surface-enhanced Raman scattering (SERS) of adsorbates on metal surfaces. The long-ra...

1992 Journal of Physics Condensed Matter 1423 citations

Publication Info

Year
2016
Type
article
Volume
93
Issue
2
Citations
11
Access
Closed

External Links

Social Impact

Social media, news, blog, policy document mentions

Citation Metrics

11
OpenAlex

Cite This

Shilin Hu, Jing Chen, Xiaolei Hao et al. (2016). Effect of low-energy electron interference on strong-field molecular ionization. Physical review. A/Physical review, A , 93 (2) . https://doi.org/10.1103/physreva.93.023424

Identifiers

DOI
10.1103/physreva.93.023424