Abstract

Abstract The production of solar fuel through photocatalytic water splitting and CO 2 reduction using photocatalysts has attracted considerable attention owing to the global energy shortage and growing environmental problems. During the past few years, many studies have demonstrated that graphene can markedly enhance the efficiency of photocatalysts for solar‐fuel generation because of its unique 2D conjugated structure and electronic properties. Herein we summarize the recent advances in the application of graphene‐based photocatalysts for solar‐fuel production, including CO 2 reduction to hydrocarbon fuel and water splitting to H 2 . A brief overview of the fundamental principles for splitting of water and reduction of CO 2 is given. The different roles of graphene in these graphene‐based photocatalysts for improving photocatalytic performance are discussed. Finally, the perspectives on the challenges and opportunities for future research in this promising area are also presented.

Keywords

Solar fuelGraphenePhotocatalysisEconomic shortageMaterials scienceSolar energyNanotechnologyWater splittingReduction (mathematics)Fuel cellsProcess engineeringEnvironmental scienceCatalysisChemical engineeringEngineeringChemistry

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Publication Info

Year
2015
Type
review
Volume
54
Issue
39
Pages
11350-11366
Citations
764
Access
Closed

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Cite This

Quanjun Xiang, Bei Cheng, Jiaguo Yu (2015). Graphene‐Based Photocatalysts for Solar‐Fuel Generation. Angewandte Chemie International Edition , 54 (39) , 11350-11366. https://doi.org/10.1002/anie.201411096

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DOI
10.1002/anie.201411096