Isolated Ni single atoms in graphene nanosheets for high-performance CO2 reduction

Kun Jiang; Samira Siahrostami; Tingting Zheng; Yongfeng Hu; Sooyeon Hwang; Eli Stavitski; Yande Peng; James J. Dynes; Mehash Gangisetty; Dong Su; Klaus Attenkofer; Haotian Wang

doi:10.1039/c7ee03245e

Abstract

High-performance electrocatalytic CO2 reduction to CO using Ni single-atom catalyst in an anion membrane electrode assembly.

Keywords

GrapheneReduction (mathematics)Materials scienceCatalysisElectrodeIonAtom (system on chip)NanotechnologyChemistryPhysical chemistryComputer science

Affiliated Institutions

Related Publications

Atomically dispersed Fe 3+ sites catalyze efficient CO 2 electroreduction to CO

Jun Gu , Chia‐Shuo Hsu , Lichen Bai +2 more

Three's a charm for iron and CO 2 Large-scale electrochemical reduction of CO 2 to CO could be a promising first step in sustainable conversion of the greenhouse gas to commodit...

2019 Science 1518 citations

Design of Single-Atom Co–N5 Catalytic Site: A Robust Electrocatalyst for CO2 Reduction with Nearly 100% CO Selectivity and Remarkable Stability

Yuan Pan , Rui Lin , Yinjuan Chen +19 more

We develop an N-coordination strategy to design a robust CO2 reduction reaction (CO2RR) electrocatalyst with atomically dispersed Co-N5 site anc...

2018 Journal of the American Chemical Society 1155 citations

Enhanced Nitrate-to-Ammonia Activity on Copper–Nickel Alloys via Tuning of Intermediate Adsorption

Yuhang Wang , Aoni Xu , Ziyun Wang +14 more

Electrochemical conversion of nitrate (NO3-) into ammonia (NH3) recycles nitrogen and offers a route to the production of NH3, which ...

2020 Journal of the American Chemical Society 1194 citations

Recent Advances and Challenges of Electrocatalytic N2Reduction to Ammonia

Shane T. Jackowski , Faezeh Habibzadeh , Mona Maleka Ashtiani +5 more

Global ammonia production reached 175 million metric tons in 2016, 90% of which is produced from high purity N2 and H2 gases at high temperatures and press...

2020 Chemical Reviews 1166 citations

Homogeneously Catalyzed Electroreduction of Carbon Dioxide—Methods, Mechanisms, and Catalysts

Robert Francke , Benjamin Schille , Michael Roemelt

The utilization of CO2 via electrochemical reduction constitutes a promising approach toward production of value-added chemicals or fuels using intermittent renewable...

2018 Chemical Reviews 1103 citations

Publication Info

Year: 2018
Type: article
Volume: 11
Issue: 4
Pages: 893-903
Citations: 974
Access: Closed

External Links

View on DOI.org

Social Impact

Altmetric

Isolated Ni single atoms in graphene nanosheets for high-performance CO2 reduction

PlumX Metrics

Social media, news, blog, policy document mentions

Citation Metrics

974

OpenAlex

Cite This

APA Style

                            
                                
                                    Kun Jiang, 
                                
                                    Samira Siahrostami, 
                                
                                    Tingting Zheng
                                
                                et al.
                            
                            (2018). 
                            Isolated Ni single atoms in graphene nanosheets for high-performance CO<sub>2</sub> reduction. 
                            Energy & Environmental Science
                            , 11
                            (4)
                            , 893-903.
                            https://doi.org/10.1039/c7ee03245e
                        

Identifiers

DOI: 10.1039/c7ee03245e

Isolated Ni single atoms in graphene nanosheets for high-performance CO<sub>2</sub> reduction